Initial estimates 207.236 133.423 32.015 20.256 BISECT FAILED BISECT FAILED Srt 0.01341 Gat 0.00000 Gbt 0.00000 Likelihood -1817.278 SSQ 81.535 AL -1898.813 Srt 0.00156 Gat 0.20838 Gbt 7.69473 Likelihood -2421.466 SSQ 305.128 AL -2726.594 Srt 0.00107 Gat 0.33952 Gbt 14.78123 Likelihood -2485.502 SSQ 422.929 AL -2908.431 Srt 0.00103 Gat 0.35670 Gbt 15.73609 Likelihood -2496.868 SSQ 450.246 AL -2947.114 Srt 0.00103 Gat 0.35830 Gbt 15.82499 Likelihood -2498.039 SSQ 457.667 AL -2955.706 Srt 0.00103 Gat 0.35844 Gbt 15.83294 Likelihood -2498.146 SSQ 459.302 AL -2957.448 Srt 0.00103 Gat 0.35845 Gbt 15.83365 Likelihood -2498.183 SSQ 459.677 AL -2957.859 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.202 SSQ 459.802 AL -2958.004 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.212 SSQ 459.866 AL -2958.078 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.217 SSQ 459.908 AL -2958.125 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.219 SSQ 459.937 AL -2958.157 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.220 SSQ 459.957 AL -2958.178 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.221 SSQ 459.971 AL -2958.192 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.221 SSQ 459.981 AL -2958.202 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.221 SSQ 459.987 AL -2958.208 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.221 SSQ 459.991 AL -2958.212 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.221 SSQ 459.994 AL -2958.215 Srt 0.00103 Gat 0.35846 Gbt 15.83372 Likelihood -2498.221 SSQ 459.996 AL -2958.217 Data in minimization i NP Eq Q Qa Qb T X2 Sr Sa Sb Total pressure Ruff & Mugdan 1 7 F F F F 1542. 0.113 0.035 0.071 1.591 Wartenberg & Albrecht 2 16 F T T T 1555. 0.164 0.032 0.019 0.128 Fiock & Rodebush 3 9 F T T T 1279. 0.121 0.032 0.019 0.128 Deitz 4 9 F T F T 896. 0.111 0.032 0.202 0.128 Barton & Bloom 5 11 T T T T 1402. 0.141 0.032 0.019 0.128 Pugh & Barrow 6 137 T T T T 880. 0.553 0.032 0.019 0.128 Novikov & Polyachenok 7 9 F T T T 1295. 0.161 0.032 0.019 0.128 Schrier & Clark 8 31 T T T T 1300. 0.225 0.032 0.019 0.128 Kushkin et al 9 10 T F F F 1246. 0.098 0.030 0.057 0.815 Barchuk & Dubovoi 10 6 F T T F 1313. 0.144 0.032 0.019 0.583 Burylev & Mironov 11 10 T F F F 1423. 0.129 0.031 0.104 2.450 Knudsen effusion Deitz 12 6 F T F T 926. 0.026 0.032 0.279 0.128 Mayer & Wintner 13 5 F T T F 923. 0.034 0.032 0.019 1.132 Zimm & Mayer 14 21 F F F F 766. 0.708 0.091 0.056 0.404 Bradley & Volans 1 15 14 F T T T 782. 0.220 0.032 0.019 0.128 Bradley & Volans 2 16 7 F T T T 812. 0.120 0.032 0.019 0.128 Bradley & Volans 3 17 6 F T T T 826. 0.101 0.032 0.019 0.128 Miller & Kusch 18 10 F T F T 924. 0.107 0.032 0.376 0.128 Nesmeyanov & Sazonov 19 7 F T T F 810. 0.199 0.032 0.019 0.565 Ewing & Stern 20 24 F F F F 901. 0.201 0.021 0.086 0.426 Kawano & Kenpo 1 21 11 F F F F 775. 0.337 0.041 0.356 0.827 Kawano & Kenpo 2 22 11 F T F T 780. 0.314 0.032 0.321 0.128 Kawano & Kenpo 3 23 10 F T F T 774. 0.289 0.032 0.274 0.128 van der Kemp et al 24 17 F F F F 899. 0.173 0.155 0.056 1.830 Transpiration Naryshkin 25 3 F F F F 1102. 0.096 0.049 0.139 0.666 Treadwell & Werner 26 13 F F F F 933. 0.211 0.018 0.206 0.752 Barton & Bloom 27 7 F T T T 1385. 0.099 0.032 0.019 0.128 Schrier & Clark 28 10 F T T T 1274. 0.130 0.032 0.019 0.128 Murgulescu & Marta 29 23 F T T T 1422. 0.076 0.032 0.019 0.128 00:01:22 Iteration 1 WORK 0.0000029 36. 5.8 0.0000000 11. INFER = 1 IER = 0 206.803 133.041 37.158 24.454 Likelihood -2504.269 SSQ 453.948 AL -2958.217 Srt 0.00101 Gat 0.30166 Gbt 11.40174 Likelihood -2505.380 SSQ 463.746 AL -2969.126 Srt 0.00102 Gat 0.29796 Gbt 11.25424 Likelihood -2505.442 SSQ 460.188 AL -2965.631 Srt 0.00102 Gat 0.29768 Gbt 11.24314 Likelihood -2505.447 SSQ 459.941 AL -2965.388 Srt 0.00102 Gat 0.29766 Gbt 11.24229 Likelihood -2505.449 SSQ 459.946 AL -2965.395 Srt 0.00102 Gat 0.29765 Gbt 11.24223 Likelihood -2505.450 SSQ 459.963 AL -2965.413 Srt 0.00102 Gat 0.29765 Gbt 11.24222 Likelihood -2505.450 SSQ 459.975 AL -2965.425 Srt 0.00102 Gat 0.29765 Gbt 11.24222 Likelihood -2505.450 SSQ 459.984 AL -2965.434 Srt 0.00102 Gat 0.29765 Gbt 11.24222 Likelihood -2505.450 SSQ 459.989 AL -2965.439 Convergence 0.199136255149317 00:20:27 Iteration 2 WORK 0.0000319 23. 4.2 0.0000154 6. INFER = 1 IER = 0 206.782 133.034 37.714 24.829 Likelihood -2505.555 SSQ 459.884 AL -2965.439 Srt 0.00102 Gat 0.29677 Gbt 11.45334 Likelihood -2505.571 SSQ 460.126 AL -2965.697 Srt 0.00102 Gat 0.29671 Gbt 11.45093 Likelihood -2505.572 SSQ 459.999 AL -2965.571 Srt 0.00102 Gat 0.29671 Gbt 11.45075 Likelihood -2505.572 SSQ 459.989 AL -2965.561 Srt 0.00102 Gat 0.29671 Gbt 11.45074 Likelihood -2505.572 SSQ 459.992 AL -2965.563 Convergence 0.263702522846083D-001 00:32:08 Iteration 3 WORK 0.0000062 23. 4.9 0.0000098 6. INFER = 1 IER = 0 206.775 133.030 37.816 24.902 Likelihood -2505.575 SSQ 459.989 AL -2965.563 Srt 0.00102 Gat 0.29663 Gbt 11.51192 Likelihood -2505.575 SSQ 460.011 AL -2965.586 Srt 0.00102 Gat 0.29663 Gbt 11.51198 Likelihood -2505.575 SSQ 459.997 AL -2965.572 Convergence 0.396854360397045D-002 00:43:19 Iteration 4 WORK 0.0000028 27. 5.7 0.0000113 6. INFER = 1 IER = 0 206.773 133.028 37.836 24.917 Likelihood -2505.575 SSQ 459.997 AL -2965.572 Srt 0.00102 Gat 0.29661 Gbt 11.52611 Likelihood -2505.575 SSQ 459.999 AL -2965.574 Convergence 0.786295536610809D-003 The norm of the gradient 0.0000028 The number of function evaluation 27. The number of significant digits in parameters 5.7 The MARQUARDT scaling parameter 0.0000113 The number of iteration 6. INFER = 1 IER = 0 DelH1 DelS1 DelH2 DelS2 206.773 133.028 37.836 24.917 Sum of squares 459.9991 Number of points 460 Average standard deviation 1.0044 LINV3P - IER 0 Parameter sqrt(Cii) 206.77 0.41 133.03 0.50 37.84 2.14 24.92 1.95 Correlation matrix 1.000 0.970 1.000 -0.631 -0.491 1.000 -0.836 -0.766 0.923 1.000 Data used in minimization i NP Eq Q Qa Qb T X2 Sr Sa Sb Total pressure Ruff & Mugdan 1 7 F F F F 1542. 0.113 0.035 0.084 1.496 Wartenberg & Albrecht 2 16 F T T T 1555. 0.164 0.032 0.017 0.109 Fiock & Rodebush 3 9 F T T T 1279. 0.121 0.032 0.017 0.109 Deitz 4 9 F T F T 896. 0.111 0.032 0.191 0.109 Barton & Bloom 5 11 T T T T 1402. 0.141 0.032 0.017 0.109 Pugh & Barrow 6 137 T T T T 880. 0.553 0.032 0.017 0.109 Novikov & Polyachenok 7 9 F T T T 1295. 0.161 0.032 0.017 0.109 Schrier & Clark 8 31 T T T T 1300. 0.225 0.032 0.017 0.109 Kushkin et al 9 10 T F F F 1246. 0.098 0.030 0.061 0.927 Barchuk & Dubovoi 10 6 F T T F 1313. 0.144 0.032 0.017 0.468 Burylev & Mironov 11 10 T F F F 1423. 0.129 0.031 0.097 2.345 Knudsen effusion Deitz 12 6 F T F T 926. 0.026 0.032 0.256 0.109 Mayer & Wintner 13 5 F T T F 923. 0.034 0.032 0.017 1.217 Zimm & Mayer 14 21 F F F F 766. 0.708 0.092 0.057 0.288 Bradley & Volans 1 15 14 F T T T 782. 0.220 0.032 0.017 0.109 Bradley & Volans 2 16 7 F T T T 812. 0.120 0.032 0.017 0.109 Bradley & Volans 3 17 6 F T T T 826. 0.101 0.032 0.017 0.109 Miller & Kusch 18 10 F T F T 924. 0.107 0.032 0.399 0.109 Nesmeyanov & Sazonov 19 7 F T T F 810. 0.199 0.032 0.017 0.451 Ewing & Stern 20 24 F F F F 901. 0.201 0.021 0.107 0.507 Kawano & Kenpo 1 21 11 F F F F 775. 0.337 0.040 0.353 0.712 Kawano & Kenpo 2 22 11 F T F T 780. 0.314 0.032 0.318 0.109 Kawano & Kenpo 3 23 10 F T F T 774. 0.289 0.032 0.272 0.109 van der Kemp et al 24 17 F F F F 899. 0.173 0.155 0.027 1.913 Transpiration Naryshkin 25 3 F F F F 1102. 0.096 0.050 0.162 0.861 Treadwell & Werner 26 13 F F F F 933. 0.211 0.018 0.173 0.721 Barton & Bloom 27 7 F T T T 1385. 0.099 0.032 0.017 0.109 Schrier & Clark 28 10 F T T T 1274. 0.130 0.032 0.017 0.109 Murgulescu & Marta 29 23 F T T T 1422. 0.076 0.032 0.017 0.109 ********************************************** ********************************************** Initial estimates 207.150 133.030 26.257 14.483 BISECT FAILED Srt 0.01588 Gat 0.25929 Gbt 0.00000 Likelihood -1712.998 SSQ 82.009 AL -1795.007 Srt 0.00204 Gat 2.66670 Gbt 10.85458 Likelihood -2338.033 SSQ 253.744 AL -2591.777 Srt 0.00113 Gat 4.91877 Gbt 28.95884 Likelihood -2441.846 SSQ 408.087 AL -2849.933 Srt 0.00104 Gat 5.32481 Gbt 32.48588 Likelihood -2454.519 SSQ 448.421 AL -2902.940 Srt 0.00104 Gat 5.36765 Gbt 32.86063 Likelihood -2455.710 SSQ 457.624 AL -2913.334 Srt 0.00103 Gat 5.37185 Gbt 32.89745 Likelihood -2455.782 SSQ 459.458 AL -2915.240 Srt 0.00103 Gat 5.37226 Gbt 32.90104 Likelihood -2455.793 SSQ 459.812 AL -2915.605 Srt 0.00103 Gat 5.37230 Gbt 32.90139 Likelihood -2455.797 SSQ 459.905 AL -2915.701 Srt 0.00103 Gat 5.37231 Gbt 32.90142 Likelihood -2455.799 SSQ 459.941 AL -2915.740 Srt 0.00103 Gat 5.37231 Gbt 32.90143 Likelihood -2455.799 SSQ 459.961 AL -2915.761 Srt 0.00103 Gat 5.37231 Gbt 32.90143 Likelihood -2455.800 SSQ 459.974 AL -2915.774 Srt 0.00103 Gat 5.37231 Gbt 32.90143 Likelihood -2455.800 SSQ 459.983 AL -2915.783 Srt 0.00103 Gat 5.37231 Gbt 32.90143 Likelihood -2455.800 SSQ 459.988 AL -2915.788 Srt 0.00103 Gat 5.37231 Gbt 32.90143 Likelihood -2455.800 SSQ 459.992 AL -2915.792 Srt 0.00103 Gat 5.37231 Gbt 32.90143 Likelihood -2455.800 SSQ 459.995 AL -2915.795 Srt 0.00103 Gat 5.37231 Gbt 32.90143 Likelihood -2455.800 SSQ 459.997 AL -2915.797 Data in minimization i NP Eq Q Qa Qb T X2 Sr Sa Sb Total pressure Ruff & Mugdan 1 7 F F F F 1542. 0.113 0.036 0.010 1.691 Wartenberg & Albrecht 2 16 F T T T 1555. 0.164 0.032 0.075 0.184 Fiock & Rodebush 3 9 F T T T 1279. 0.121 0.032 0.075 0.184 Deitz 4 9 F T F T 896. 0.111 0.032 0.177 0.184 Barton & Bloom 5 11 T T T T 1402. 0.141 0.032 0.075 0.184 Pugh & Barrow 6 137 T T T T 880. 0.553 0.032 0.075 0.184 Novikov & Polyachenok 7 9 F T T T 1295. 0.161 0.032 0.075 0.184 Schrier & Clark 8 31 T T T T 1300. 0.225 0.032 0.075 0.184 Kushkin et al 9 10 T F F F 1246. 0.098 0.030 0.127 0.646 Barchuk & Dubovoi 10 6 F T T F 1313. 0.144 0.032 0.075 0.736 Burylev & Mironov 11 10 T F F F 1423. 0.129 0.031 0.188 2.575 Knudsen effusion Deitz 12 6 F T F T 926. 0.026 0.032 0.254 0.184 Mayer & Wintner 13 5 F T T F 923. 0.034 0.032 0.075 1.270 Zimm & Mayer 14 21 F F F F 766. 0.708 0.090 0.074 0.392 Bradley & Volans 1 15 14 F T T T 782. 0.220 0.032 0.075 0.184 Bradley & Volans 2 16 7 F T T T 812. 0.120 0.032 0.075 0.184 Bradley & Volans 3 17 6 F T T T 826. 0.101 0.032 0.075 0.184 Miller & Kusch 18 10 F T F T 924. 0.107 0.032 0.402 0.184 Nesmeyanov & Sazonov 19 7 F T T F 810. 0.199 0.032 0.075 0.529 Ewing & Stern 20 24 F F F F 901. 0.201 0.022 0.109 0.516 Kawano & Kenpo 1 21 11 F F F F 775. 0.337 0.041 0.340 0.815 Kawano & Kenpo 2 22 11 F T F T 780. 0.314 0.032 0.306 0.184 Kawano & Kenpo 3 23 10 F T F T 774. 0.289 0.032 0.259 0.184 van der Kemp et al 24 17 F F F F 899. 0.173 0.155 0.024 1.935 Transpiration Naryshkin 25 3 F F F F 1102. 0.096 0.049 0.201 0.263 Treadwell & Werner 26 13 F F F F 933. 0.211 0.018 0.182 0.581 Barton & Bloom 27 7 F T T T 1385. 0.099 0.032 0.075 0.184 Schrier & Clark 28 10 F T T T 1274. 0.130 0.032 0.075 0.184 Murgulescu & Marta 29 23 F T T T 1422. 0.076 0.032 0.075 0.184 01:00:01 Iteration 1 WORK 0.0000069 32. 5.1 0.0000001 11. INFER = 1 IER = 0 205.837 131.572 36.844 25.607 Likelihood -2471.526 SSQ 444.271 AL -2915.797 Srt 0.00098 Gat 1.53633 Gbt 16.81617 Likelihood -2482.456 SSQ 473.990 AL -2956.446 Srt 0.00102 Gat 1.47134 Gbt 15.98380 Likelihood -2482.864 SSQ 460.830 AL -2943.694 Srt 0.00103 Gat 1.46601 Gbt 15.91592 Likelihood -2482.885 SSQ 459.894 AL -2942.779 Srt 0.00103 Gat 1.46555 Gbt 15.91014 Likelihood -2482.893 SSQ 459.881 AL -2942.774 Srt 0.00103 Gat 1.46551 Gbt 15.90965 Likelihood -2482.897 SSQ 459.918 AL -2942.815 Srt 0.00103 Gat 1.46551 Gbt 15.90961 Likelihood -2482.899 SSQ 459.945 AL -2942.844 Srt 0.00103 Gat 1.46551 Gbt 15.90960 Likelihood -2482.900 SSQ 459.963 AL -2942.863 Srt 0.00103 Gat 1.46551 Gbt 15.90960 Likelihood -2482.900 SSQ 459.975 AL -2942.875 Srt 0.00103 Gat 1.46551 Gbt 15.90960 Likelihood -2482.900 SSQ 459.983 AL -2942.884 Srt 0.00103 Gat 1.46551 Gbt 15.90960 Likelihood -2482.900 SSQ 459.989 AL -2942.889 Convergence 0.751053942211165 01:17:59 Iteration 2 WORK 0.0000510 23. 4.3 0.0000098 6. INFER = 1 IER = 0 206.024 131.929 38.101 26.537 Likelihood -2489.619 SSQ 453.270 AL -2942.889 Srt 0.00100 Gat 0.52803 Gbt 13.31193 Likelihood -2497.197 SSQ 468.005 AL -2965.203 Srt 0.00102 Gat 0.51156 Gbt 12.89234 Likelihood -2497.801 SSQ 460.066 AL -2957.866 Srt 0.00102 Gat 0.51025 Gbt 12.85911 Likelihood -2497.863 SSQ 459.829 AL -2957.692 Srt 0.00102 Gat 0.51014 Gbt 12.85641 Likelihood -2497.869 SSQ 459.935 AL -2957.803 Srt 0.00102 Gat 0.51014 Gbt 12.85619 Likelihood -2497.869 SSQ 459.980 AL -2957.849 Srt 0.00102 Gat 0.51013 Gbt 12.85617 Likelihood -2497.869 SSQ 459.994 AL -2957.863 Convergence 0.426624139953977 01:30:09 Iteration 3 WORK 0.0000676 23. 4.1 0.0000338 6. INFER = 1 IER = 0 206.647 132.853 38.083 25.361 Likelihood -2503.432 SSQ 454.431 AL -2957.863 Srt 0.00101 Gat 0.30587 Gbt 11.84430 Likelihood -2505.333 SSQ 464.551 AL -2969.884 Srt 0.00102 Gat 0.30073 Gbt 11.64473 Likelihood -2505.428 SSQ 460.221 AL -2965.649 Srt 0.00102 Gat 0.30035 Gbt 11.62982 Likelihood -2505.433 SSQ 459.974 AL -2965.406 Srt 0.00102 Gat 0.30032 Gbt 11.62869 Likelihood -2505.433 SSQ 459.981 AL -2965.414 Srt 0.00102 Gat 0.30032 Gbt 11.62861 Likelihood -2505.433 SSQ 459.991 AL -2965.424 Convergence 0.211950623309562 01:42:06 Iteration 4 WORK 0.0000123 23. 5.1 0.0000098 6. INFER = 1 IER = 0 206.762 133.014 37.880 24.966 Likelihood -2505.565 SSQ 459.860 AL -2965.424 Srt 0.00102 Gat 0.29671 Gbt 11.56203 Likelihood -2505.574 SSQ 460.100 AL -2965.674 Srt 0.00102 Gat 0.29658 Gbt 11.55699 Likelihood -2505.575 SSQ 460.004 AL -2965.578 Srt 0.00102 Gat 0.29657 Gbt 11.55661 Likelihood -2505.575 SSQ 459.998 AL -2965.572 Convergence 0.188728553127886D-001 01:53:32 Iteration 5 WORK 0.0000025 23. 5.7 0.0000098 6. INFER = 1 IER = 0 206.771 133.026 37.849 24.927 Likelihood -2505.575 SSQ 459.997 AL -2965.572 Srt 0.00102 Gat 0.29659 Gbt 11.53625 Likelihood -2505.575 SSQ 459.996 AL -2965.571 Convergence 0.142581990553290D-002 02:04:28 Iteration 6 WORK 0.0033046 14. 4.3 0.0025000 1. INFER = 1 IER = 0 206.772 133.027 37.847 24.926 Likelihood -2505.575 SSQ 459.996 AL -2965.571 Srt 0.00102 Gat 0.29661 Gbt 11.53380 Likelihood -2505.575 SSQ 459.998 AL -2965.573 Convergence 0.203072292805761D-003 The norm of the gradient 0.0033046 The number of function evaluation 14. The number of significant digits in parameters 4.3 The MARQUARDT scaling parameter 0.0025000 The number of iteration 1. INFER = 1 IER = 0 DelH1 DelS1 DelH2 DelS2 206.772 133.027 37.847 24.926 Sum of squares 459.9979 Number of points 460 Average standard deviation 1.0044 LINV3P - IER 0 Parameter sqrt(Cii) 206.77 0.41 133.03 0.50 37.85 2.14 24.93 1.95 Correlation matrix 1.000 0.970 1.000 -0.631 -0.491 1.000 -0.836 -0.766 0.923 1.000 Data used in minimization i NP Eq Q Qa Qb T X2 Sr Sa Sb Total pressure Ruff & Mugdan 1 7 F F F F 1542. 0.113 0.035 0.084 1.496 Wartenberg & Albrecht 2 16 F T T T 1555. 0.164 0.032 0.017 0.109 Fiock & Rodebush 3 9 F T T T 1279. 0.121 0.032 0.017 0.109 Deitz 4 9 F T F T 896. 0.111 0.032 0.191 0.109 Barton & Bloom 5 11 T T T T 1402. 0.141 0.032 0.017 0.109 Pugh & Barrow 6 137 T T T T 880. 0.553 0.032 0.017 0.109 Novikov & Polyachenok 7 9 F T T T 1295. 0.161 0.032 0.017 0.109 Schrier & Clark 8 31 T T T T 1300. 0.225 0.032 0.017 0.109 Kushkin et al 9 10 T F F F 1246. 0.098 0.030 0.061 0.928 Barchuk & Dubovoi 10 6 F T T F 1313. 0.144 0.032 0.017 0.467 Burylev & Mironov 11 10 T F F F 1423. 0.129 0.031 0.097 2.345 Knudsen effusion Deitz 12 6 F T F T 926. 0.026 0.032 0.256 0.109 Mayer & Wintner 13 5 F T T F 923. 0.034 0.032 0.017 1.218 Zimm & Mayer 14 21 F F F F 766. 0.708 0.092 0.057 0.288 Bradley & Volans 1 15 14 F T T T 782. 0.220 0.032 0.017 0.109 Bradley & Volans 2 16 7 F T T T 812. 0.120 0.032 0.017 0.109 Bradley & Volans 3 17 6 F T T T 826. 0.101 0.032 0.017 0.109 Miller & Kusch 18 10 F T F T 924. 0.107 0.032 0.399 0.109 Nesmeyanov & Sazonov 19 7 F T T F 810. 0.199 0.032 0.017 0.451 Ewing & Stern 20 24 F F F F 901. 0.201 0.021 0.107 0.507 Kawano & Kenpo 1 21 11 F F F F 775. 0.337 0.040 0.353 0.712 Kawano & Kenpo 2 22 11 F T F T 780. 0.314 0.032 0.318 0.109 Kawano & Kenpo 3 23 10 F T F T 774. 0.289 0.032 0.272 0.109 van der Kemp et al 24 17 F F F F 899. 0.173 0.155 0.027 1.914 Transpiration Naryshkin 25 3 F F F F 1102. 0.096 0.050 0.162 0.861 Treadwell & Werner 26 13 F F F F 933. 0.211 0.018 0.173 0.720 Barton & Bloom 27 7 F T T T 1385. 0.099 0.032 0.017 0.109 Schrier & Clark 28 10 F T T T 1274. 0.130 0.032 0.017 0.109 Murgulescu & Marta 29 23 F T T T 1422. 0.076 0.032 0.017 0.109 ********************************************** ********************************************** Initial estimates 206.466 132.139 23.645 16.252 BISECT FAILED Srt 0.01923 Gat 0.10605 Gbt 0.00000 Likelihood -1710.439 SSQ 93.790 AL -1804.229 Srt 0.00245 Gat 1.64874 Gbt 38.13300 Likelihood -2308.751 SSQ 249.274 AL -2558.024 Srt 0.00120 Gat 3.53278 Gbt 110.19670 Likelihood -2428.996 SSQ 398.399 AL -2827.395 Srt 0.00106 Gat 4.00181 Gbt 128.60408 Likelihood -2448.291 SSQ 444.747 AL -2893.038 Srt 0.00105 Gat 4.06091 Gbt 130.93011 Likelihood -2450.832 SSQ 456.842 AL -2907.674 Srt 0.00104 Gat 4.06754 Gbt 131.19115 Likelihood -2450.956 SSQ 459.443 AL -2910.399 Srt 0.00104 Gat 4.06828 Gbt 131.22004 Likelihood -2450.960 SSQ 459.902 AL -2910.862 Srt 0.00104 Gat 4.06836 Gbt 131.22323 Likelihood -2450.960 SSQ 459.982 AL -2910.942 Srt 0.00104 Gat 4.06837 Gbt 131.22359 Likelihood -2450.960 SSQ 459.997 AL -2910.957 Data in minimization i NP Eq Q Qa Qb T X2 Sr Sa Sb Total pressure Ruff & Mugdan 1 7 F F F F 1542. 0.113 0.035 0.013 1.972 Wartenberg & Albrecht 2 16 F T T T 1555. 0.164 0.032 0.065 0.370 Fiock & Rodebush 3 9 F T T T 1279. 0.121 0.032 0.065 0.370 Deitz 4 9 F T F T 896. 0.111 0.032 0.263 0.370 Barton & Bloom 5 11 T T T T 1402. 0.141 0.032 0.065 0.370 Pugh & Barrow 6 137 T T T T 880. 0.553 0.032 0.065 0.370 Novikov & Polyachenok 7 9 F T T T 1295. 0.161 0.032 0.065 0.370 Schrier & Clark 8 31 T T T T 1300. 0.225 0.032 0.065 0.370 Kushkin et al 9 10 T F F F 1246. 0.098 0.030 0.052 0.371 Barchuk & Dubovoi 10 6 F T T F 1313. 0.144 0.032 0.065 0.988 Burylev & Mironov 11 10 T F F F 1423. 0.129 0.031 0.138 2.839 Knudsen effusion Deitz 12 6 F T F T 926. 0.026 0.032 0.378 0.370 Mayer & Wintner 13 5 F T T F 923. 0.034 0.032 0.065 1.033 Zimm & Mayer 14 21 F F F F 766. 0.708 0.090 0.000 0.522 Bradley & Volans 1 15 14 F T T T 782. 0.220 0.032 0.065 0.370 Bradley & Volans 2 16 7 F T T T 812. 0.120 0.032 0.065 0.370 Bradley & Volans 3 17 6 F T T T 826. 0.101 0.032 0.065 0.370 Miller & Kusch 18 10 F T F T 924. 0.107 0.032 0.278 0.370 Nesmeyanov & Sazonov 19 7 F T T F 810. 0.199 0.032 0.065 0.694 Ewing & Stern 20 24 F F F F 901. 0.201 0.022 0.009 0.332 Kawano & Kenpo 1 21 11 F F F F 775. 0.337 0.041 0.431 0.956 Kawano & Kenpo 2 22 11 F T F T 780. 0.314 0.032 0.397 0.370 Kawano & Kenpo 3 23 10 F T F T 774. 0.289 0.032 0.349 0.370 van der Kemp et al 24 17 F F F F 899. 0.173 0.155 0.159 1.737 Transpiration Naryshkin 25 3 F F F F 1102. 0.096 0.041 0.023 0.000 Treadwell & Werner 26 13 F F F F 933. 0.211 0.018 0.346 0.786 Barton & Bloom 27 7 F T T T 1385. 0.099 0.032 0.065 0.370 Schrier & Clark 28 10 F T T T 1274. 0.130 0.032 0.065 0.370 Murgulescu & Marta 29 23 F T T T 1422. 0.076 0.032 0.065 0.370 02:13:06 Iteration 1 WORK 0.0000078 36. 5.1 0.0000000 11. INFER = 1 IER = 0 206.142 131.765 26.806 19.189 Likelihood -2457.489 SSQ 453.468 AL -2910.957 Srt 0.00102 Gat 2.85596 Gbt 101.32233 Likelihood -2459.256 SSQ 466.702 AL -2925.958 Srt 0.00104 Gat 2.79326 Gbt 98.52119 Likelihood -2459.393 SSQ 460.524 AL -2919.917 Srt 0.00104 Gat 2.78655 Gbt 98.22149 Likelihood -2459.399 SSQ 459.983 AL -2919.382 Srt 0.00104 Gat 2.78582 Gbt 98.18875 Likelihood -2459.400 SSQ 459.963 AL -2919.363 Srt 0.00104 Gat 2.78574 Gbt 98.18516 Likelihood -2459.400 SSQ 459.976 AL -2919.376 Srt 0.00104 Gat 2.78573 Gbt 98.18477 Likelihood -2459.400 SSQ 459.986 AL -2919.386 Srt 0.00104 Gat 2.78573 Gbt 98.18473 Likelihood -2459.400 SSQ 459.991 AL -2919.391 Convergence 0.354915196311756 02:31:45 Iteration 2 WORK 0.0000014 39. 5.8 0.0000001 10. INFER = 1 IER = 0 206.392 132.243 27.680 19.165 Likelihood -2461.460 SSQ 457.931 AL -2919.391 Srt 0.00102 Gat 2.36791 Gbt 69.05864 Likelihood -2464.052 SSQ 462.868 AL -2926.920 Srt 0.00104 Gat 2.32900 Gbt 67.56241 Likelihood -2464.316 SSQ 459.942 AL -2924.258 Srt 0.00104 Gat 2.32491 Gbt 67.40516 Likelihood -2464.341 SSQ 459.813 AL -2924.154 Srt 0.00104 Gat 2.32447 Gbt 67.38838 Likelihood -2464.348 SSQ 459.877 AL -2924.225 Srt 0.00104 Gat 2.32442 Gbt 67.38658 Likelihood -2464.350 SSQ 459.923 AL -2924.274 Srt 0.00104 Gat 2.32442 Gbt 67.38639 Likelihood -2464.352 SSQ 459.951 AL -2924.302 Srt 0.00104 Gat 2.32442 Gbt 67.38637 Likelihood -2464.352 SSQ 459.968 AL -2924.320 Srt 0.00104 Gat 2.32442 Gbt 67.38637 Likelihood -2464.353 SSQ 459.978 AL -2924.331 Srt 0.00104 Gat 2.32442 Gbt 67.38637 Likelihood -2464.353 SSQ 459.986 AL -2924.338 Srt 0.00104 Gat 2.32442 Gbt 67.38637 Likelihood -2464.353 SSQ 459.990 AL -2924.343 Convergence 0.197141992133564 02:52:20 Iteration 3 WORK 0.0000017 36. 5.7 0.0000000 11. INFER = 1 IER = 0 206.433 132.589 31.380 21.090 Likelihood -2470.360 SSQ 453.983 AL -2924.343 Srt 0.00100 Gat 1.54471 Gbt 26.89174 Likelihood -2477.540 SSQ 466.901 AL -2944.442 Srt 0.00103 Gat 1.49513 Gbt 25.61151 Likelihood -2478.176 SSQ 460.218 AL -2938.394 Srt 0.00104 Gat 1.49044 Gbt 25.49075 Likelihood -2478.219 SSQ 459.773 AL -2937.992 Srt 0.00104 Gat 1.48998 Gbt 25.47899 Likelihood -2478.238 SSQ 459.813 AL -2938.050 Srt 0.00104 Gat 1.48994 Gbt 25.47785 Likelihood -2478.247 SSQ 459.870 AL -2938.117 Srt 0.00104 Gat 1.48994 Gbt 25.47773 Likelihood -2478.252 SSQ 459.911 AL -2938.163 Srt 0.00104 Gat 1.48993 Gbt 25.47772 Likelihood -2478.254 SSQ 459.940 AL -2938.193 Srt 0.00104 Gat 1.48993 Gbt 25.47772 Likelihood -2478.255 SSQ 459.959 AL -2938.214 Srt 0.00104 Gat 1.48993 Gbt 25.47772 Likelihood -2478.255 SSQ 459.972 AL -2938.228 Srt 0.00104 Gat 1.48993 Gbt 25.47772 Likelihood -2478.255 SSQ 459.981 AL -2938.237 Srt 0.00104 Gat 1.48993 Gbt 25.47772 Likelihood -2478.256 SSQ 459.988 AL -2938.243 Convergence 0.422359782270265 03:12:02 Iteration 4 WORK 0.0000105 36. 5.3 0.0000001 11. INFER = 1 IER = 0 206.350 132.650 36.686 24.527 Likelihood -2487.930 SSQ 450.313 AL -2938.243 Srt 0.00099 Gat 0.64015 Gbt 14.43034 Likelihood -2495.453 SSQ 468.207 AL -2963.660 Srt 0.00102 Gat 0.61797 Gbt 13.89477 Likelihood -2495.881 SSQ 460.328 AL -2956.209 Srt 0.00102 Gat 0.61622 Gbt 13.85272 Likelihood -2495.907 SSQ 459.837 AL -2955.744 Srt 0.00102 Gat 0.61608 Gbt 13.84932 Likelihood -2495.919 SSQ 459.858 AL -2955.777 Srt 0.00102 Gat 0.61607 Gbt 13.84904 Likelihood -2495.924 SSQ 459.901 AL -2955.825 Srt 0.00102 Gat 0.61607 Gbt 13.84902 Likelihood -2495.927 SSQ 459.932 AL -2955.859 Srt 0.00102 Gat 0.61607 Gbt 13.84902 Likelihood -2495.928 SSQ 459.954 AL -2955.882 Srt 0.00102 Gat 0.61607 Gbt 13.84902 Likelihood -2495.929 SSQ 459.969 AL -2955.898 Srt 0.00102 Gat 0.61607 Gbt 13.84902 Likelihood -2495.929 SSQ 459.979 AL -2955.908 Srt 0.00102 Gat 0.61607 Gbt 13.84902 Likelihood -2495.929 SSQ 459.986 AL -2955.915 Srt 0.00102 Gat 0.61607 Gbt 13.84902 Likelihood -2495.929 SSQ 459.991 AL -2955.920 Convergence 0.605655831687420 03:31:48 Iteration 5 WORK 0.0000035 36. 6.5 0.0000000 11. INFER = 1 IER = 0 206.584 132.852 37.983 25.213 Likelihood -2501.187 SSQ 454.733 AL -2955.920 Srt 0.00100 Gat 0.32973 Gbt 12.69459 Likelihood -2504.407 SSQ 464.763 AL -2969.170 Srt 0.00102 Gat 0.32252 Gbt 12.41711 Likelihood -2504.582 SSQ 460.223 AL -2964.805 Srt 0.00102 Gat 0.32198 Gbt 12.39642 Likelihood -2504.586 SSQ 459.956 AL -2964.542 Srt 0.00102 Gat 0.32194 Gbt 12.39485 Likelihood -2504.587 SSQ 459.958 AL -2964.545 Srt 0.00102 Gat 0.32193 Gbt 12.39473 Likelihood -2504.588 SSQ 459.971 AL -2964.559 Srt 0.00102 Gat 0.32193 Gbt 12.39472 Likelihood -2504.588 SSQ 459.981 AL -2964.568 Srt 0.00102 Gat 0.32193 Gbt 12.39472 Likelihood -2504.588 SSQ 459.987 AL -2964.575 Srt 0.00102 Gat 0.32193 Gbt 12.39472 Likelihood -2504.588 SSQ 459.991 AL -2964.579 Convergence 0.363035009621982 03:50:51 Iteration 6 WORK 0.0000099 23. 5.5 0.0000098 6. INFER = 1 IER = 0 206.740 132.998 37.898 24.990 Likelihood -2505.413 SSQ 459.166 AL -2964.579 Srt 0.00102 Gat 0.29843 Gbt 11.73472 Likelihood -2505.547 SSQ 460.885 AL -2966.431 Srt 0.00102 Gat 0.29722 Gbt 11.68634 Likelihood -2505.555 SSQ 460.043 AL -2965.598 Srt 0.00102 Gat 0.29712 Gbt 11.68269 Likelihood -2505.556 SSQ 459.990 AL -2965.545 Srt 0.00102 Gat 0.29712 Gbt 11.68242 Likelihood -2505.556 SSQ 459.990 AL -2965.546 Convergence 0.898316973075664D-001 04:02:32 Iteration 7 WORK 0.0000026 23. 5.5 0.0000098 6. INFER = 1 IER = 0 206.768 133.023 37.854 24.932 Likelihood -2505.573 SSQ 459.973 AL -2965.546 Srt 0.00102 Gat 0.29664 Gbt 11.56049 Likelihood -2505.575 SSQ 460.039 AL -2965.614 Srt 0.00102 Gat 0.29656 Gbt 11.55719 Likelihood -2505.575 SSQ 459.997 AL -2965.572 Srt 0.00102 Gat 0.29655 Gbt 11.55694 Likelihood -2505.575 SSQ 459.996 AL -2965.571 Convergence 0.109662088219620D-001 04:13:58 Iteration 8 WORK 0.0187199 10. 4.4 0.0025000 1. INFER = 1 IER = 0 206.769 133.024 37.852 24.933 Likelihood -2505.575 SSQ 459.996 AL -2965.571 Srt 0.00102 Gat 0.29662 Gbt 11.54093 Likelihood -2505.575 SSQ 460.000 AL -2965.575 Convergence 0.128001082983992D-002 04:18:33 Iteration 9 WORK 0.0116463 14. 4.2 0.0025000 1. INFER = 1 IER = 0 206.770 133.025 37.851 24.931 Likelihood -2505.575 SSQ 460.000 AL -2965.575 Srt 0.00102 Gat 0.29663 Gbt 11.53724 Likelihood -2505.575 SSQ 459.998 AL -2965.574 Convergence 0.286469252343794D-003 The norm of the gradient 0.0116463 The number of function evaluation 14. The number of significant digits in parameters 4.2 The MARQUARDT scaling parameter 0.0025000 The number of iteration 1. INFER = 1 IER = 0 DelH1 DelS1 DelH2 DelS2 206.770 133.025 37.851 24.931 Sum of squares 459.9985 Number of points 460 Average standard deviation 1.0044 LINV3P - IER 0 Parameter sqrt(Cii) 206.77 0.41 133.02 0.50 37.85 2.14 24.93 1.95 Correlation matrix 1.000 0.970 1.000 -0.631 -0.491 1.000 -0.836 -0.765 0.923 1.000 Data used in minimization i NP Eq Q Qa Qb T X2 Sr Sa Sb Total pressure Ruff & Mugdan 1 7 F F F F 1542. 0.113 0.035 0.084 1.496 Wartenberg & Albrecht 2 16 F T T T 1555. 0.164 0.032 0.017 0.109 Fiock & Rodebush 3 9 F T T T 1279. 0.121 0.032 0.017 0.109 Deitz 4 9 F T F T 896. 0.111 0.032 0.191 0.109 Barton & Bloom 5 11 T T T T 1402. 0.141 0.032 0.017 0.109 Pugh & Barrow 6 137 T T T T 880. 0.553 0.032 0.017 0.109 Novikov & Polyachenok 7 9 F T T T 1295. 0.161 0.032 0.017 0.109 Schrier & Clark 8 31 T T T T 1300. 0.225 0.032 0.017 0.109 Kushkin et al 9 10 T F F F 1246. 0.098 0.030 0.061 0.928 Barchuk & Dubovoi 10 6 F T T F 1313. 0.144 0.032 0.017 0.467 Burylev & Mironov 11 10 T F F F 1423. 0.129 0.031 0.097 2.345 Knudsen effusion Deitz 12 6 F T F T 926. 0.026 0.032 0.256 0.109 Mayer & Wintner 13 5 F T T F 923. 0.034 0.032 0.017 1.218 Zimm & Mayer 14 21 F F F F 766. 0.708 0.092 0.057 0.288 Bradley & Volans 1 15 14 F T T T 782. 0.220 0.032 0.017 0.109 Bradley & Volans 2 16 7 F T T T 812. 0.120 0.032 0.017 0.109 Bradley & Volans 3 17 6 F T T T 826. 0.101 0.032 0.017 0.109 Miller & Kusch 18 10 F T F T 924. 0.107 0.032 0.399 0.109 Nesmeyanov & Sazonov 19 7 F T T F 810. 0.199 0.032 0.017 0.451 Ewing & Stern 20 24 F F F F 901. 0.201 0.021 0.107 0.507 Kawano & Kenpo 1 21 11 F F F F 775. 0.337 0.040 0.353 0.712 Kawano & Kenpo 2 22 11 F T F T 780. 0.314 0.032 0.318 0.109 Kawano & Kenpo 3 23 10 F T F T 774. 0.289 0.032 0.272 0.109 van der Kemp et al 24 17 F F F F 899. 0.173 0.155 0.027 1.914 Transpiration Naryshkin 25 3 F F F F 1102. 0.096 0.050 0.162 0.861 Treadwell & Werner 26 13 F F F F 933. 0.211 0.018 0.173 0.720 Barton & Bloom 27 7 F T T T 1385. 0.099 0.032 0.017 0.109 Schrier & Clark 28 10 F T T T 1274. 0.130 0.032 0.017 0.109 Murgulescu & Marta 29 23 F T T T 1422. 0.076 0.032 0.017 0.109 ********************************************** ********************************************** 04:24:44 Confident limit for DelS2 SS SSlin DelH1 DelS1 DelH2 DelS2 459.998 459.998 206.77 133.02 37.85 24.93 461.055 460.998 206.42 132.64 39.84 26.88 464.406 463.998 206.08 132.25 41.87 28.83 470.358 468.998 205.73 131.88 43.95 30.78 479.217 475.998 205.41 131.53 46.11 32.72 491.268 484.998 205.11 131.22 48.37 34.67 506.738 495.998 204.86 130.98 50.78 36.62 525.716 508.998 204.69 130.86 53.42 38.57 548.024 523.998 204.66 130.91 56.40 40.52 460.941 460.998 207.11 133.41 35.89 22.98 463.605 463.998 207.45 133.79 33.96 21.04 467.732 468.998 207.78 134.16 32.05 19.09 473.086 475.998 208.10 134.51 30.15 17.14 479.450 484.998 208.41 134.86 28.26 15.19 486.626 495.998 208.70 135.19 26.38 13.24 494.437 508.998 208.99 135.52 24.50 11.29 502.723 523.998 209.27 135.82 22.63 9.35 07:33:05